Welcome. :)
Well, the thing about nVidia Surround is twofold: it requires two cards, which makes it more expensive, and they've not really updated it since it was released. If you use the 258.96 drivers that were the first officially stable Surround capable drivers, you're not missing any features from the later drivers as there aren't any new ones. Except a modified setup procedure.
While with AMD, a single card can do great, but trying to pair CrossFireX and EyeFinity can yield all sorts of headaches.
Also something that needs to be taken into consideration with nVidia Surround is the fact that you'll really need 2GB+ of VRAM, so the 'cheapest' GTX560s etc aren't the way to go. I don't know how much 2GB GTX560s cost in the US at the minute, but you'll need a pair of them if you want the nVidia route.
The AMD route is a little easier: a single 6950 (if you flash it to 6970) or a single 6970.
Then the best monitors you can afford. Three of something like the Dell U2211H or U2311H.
Actually, given the board you're using, you'll need to go the AMD route for a single card. If you want to drop the res a bit for a FPS boost, look at 1680x1050 or 1600x900 screens.
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